%0 Book
%T Hydrogen generation from the chemical energy carrier methanol: mechanistic insights into the ruthenium-catalysed dehydrogenation reaction and the implementation of a novel base-metal catalyst system
%A Vogt, Lydia Katharina
%D 2017
%C Rostock
%C Universität Rostock
%G English
%F 892902728
%O submitted by M. Sc. Lydia Katharina Vogt (née Neumann)
%O Dissertation Universität Rostock 2017
%X This thesis deals with the aqueous-phase reforming of methanol catalysed by homogeneous pincer complexes. Based on extensive kinetic experiments, spectroscopic investigations and supporting theoretical calculations, a complete mechanistic cycle could be proposed for a Ru-pincer catalyst and its methylated derivative. Furthermore, a highly stable catalyst system based on the base metal manganese was implemented for the low-temperature dehydrogenation of methanol.<eng>
%L 540
%9 theses
%9 Text
%9 Hochschulschrift
%U http://rosdok.uni-rostock.de/resolve/urn/urn:nbn:de:gbv:28-diss2017-0086-0