Unraveling property-performance relationships in CO2 hydrogenation over iron-based catalysts Yang, Qingxin , 1993- (VerfasserIn) Kondratenko, Evgenii (AkademischeR BetreuerIn) Khodakov, Andrei (AkademischeR BetreuerIn) Universität Rostock (Grad-verleihende Institution) Universität Rostock Mathematisch-Naturwissenschaftliche Fakultät (Grad-verleihende Institution) Text theses Text Hochschulschrift 2022 2022 eng electronic resourceremoteComputermedienOnline-Ressource1 Online-Ressource This thesis deals with the development of iron-based catalysts for CO2 hydrogenation to higher hydrocarbons and understanding of fundamentals relevant for activity and selectivity. The most decisive factors affecting activity and selectivity were identified by statistical approaches. The promotion effects of alkali metal promoter on CO2 hydrogenation over Fe-based catalysts were elucidated through characterization and kinetic analyses. This thesis also contributes to understanding of the interplay between physicochemical properties of promoter-free Fe-based catalyst and catalytic performance.<eng> vorgelegt von Qingxin Yang GutachterInnen: Evgenii Kondratenko (Leibniz-Institut für Katalyse e.V.) ; Andrei Khodakov (Universität Lille) Dissertation Universität Rostock 2022 540 660.2995 660 35.17 http://purl.uni-rostock.de/rosdok/id00003779 https://doi.org/10.18453/rosdok_id00003779 https://nbn-resolving.org/urn:nbn:de:gbv:28-rosdok_id00003779-6 https://d-nb.info/1293538108/34 Unraveling property-performance relationships in CO2 hydrogenation over iron-based catalysts--(DE-627)1810700574 urn:nbn:de:gbv:28-rosdok_id00003779-6 doi: 10.18453/rosdok_id00003779 oclc: 1335595197 ppn: (DE-627)1810124166