@Book{1789926815, author="Leonard, David", title="Development of 3d metal catalysts for redox reactions", year="2021", address="Rostock", abstract="Herein is reported the application of non-noble metal-based catalytic systems for the homogeneous oxidation of organic substrates using air, specifically in amines and N-heterocycles. Simple 3d metal salts have been used, in combination with N-ligands, to facilitate the oxidative cleavage of C(sp3)--C(sp3) bonds. These reactions have been studied, using spectroscopic methods, to propose plausible mechanistic pathways. We believe such deconstructive strategies can enable late-stage functionalisation of pharmaceuticals and the synthesis of drug metabolites.", school="Universit{\"a}t Rostock", note="vorgelegt von David Leonard", note="Enth{\"a}lt Zeitschriftenartikel", note="GutachterInnen: Matthias Beller (Leibniz Institute for Catalysis) ; Shoubhik Das (University of Antwerp)", note="Dissertation Universit{\"a}t Rostock 2021 Kumulative Dissertation", doi="10.18453/rosdok_id00003492", url="http://purl.uni-rostock.de/rosdok/id00003492", url="https://nbn-resolving.org/urn:nbn:de:gbv:28-rosdok_id00003492-4", url="https://d-nb.info/1293536709/34", url="https://doi.org/10.18453/rosdok_id00003492", language="English" }